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Unraveling the surface self-reconstruction of Fe-doped Ni-thiophosphate for efficient oxygen evolution reaction
- Authors
- Kirubasankar, Balakrishnan; Won, Yo Seob; Choi, Soo Ho; Kim, Jae Woo; Adofo, Laud Anim; Kim, Soo Min; Kim, Ki Kang
- Issue Date
- Jul-2023
- Publisher
- ROYAL SOC CHEMISTRY
- Citation
- CHEMICAL COMMUNICATIONS, v.59, no.60, pp 9247 - 9250
- Pages
- 4
- Journal Title
- CHEMICAL COMMUNICATIONS
- Volume
- 59
- Number
- 60
- Start Page
- 9247
- End Page
- 9250
- ISSN
- 1359-7345
1364-548X
- Abstract
- Surface self-reconstruction of oxygen evolution reaction (OER) electrocatalysts generally occurs during the electrochemical activation process. Herein, we study the surface self-reconstruction of a 2D layered Fe-doped Ni-thiophosphate (NixFe1-xPS3) nanosheet. The role of Fe in the surface self-reconstruction of NiPS3 during the OER is investigated by using an in situ Raman analysis. Formation of amorphous metal/non-metal oxide layers on the surface of NixFe1-xPS3 can efficiently act as the ultimate catalytic center for the OER.
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