Unraveling the surface self-reconstruction of Fe-doped Ni-thiophosphate for efficient oxygen evolution reaction
  • Kirubasankar, Balakrishnan
  • Won, Yo Seob
  • Choi, Soo Ho
  • Kim, Jae Woo
  • Adofo, Laud Anim
  • ... Kim, Soo Min
  • 외 1명
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초록

Surface self-reconstruction of oxygen evolution reaction (OER) electrocatalysts generally occurs during the electrochemical activation process. Herein, we study the surface self-reconstruction of a 2D layered Fe-doped Ni-thiophosphate (NixFe1-xPS3) nanosheet. The role of Fe in the surface self-reconstruction of NiPS3 during the OER is investigated by using an in situ Raman analysis. Formation of amorphous metal/non-metal oxide layers on the surface of NixFe1-xPS3 can efficiently act as the ultimate catalytic center for the OER.

키워드

HYDROGEN
제목
Unraveling the surface self-reconstruction of Fe-doped Ni-thiophosphate for efficient oxygen evolution reaction
저자
Kirubasankar, BalakrishnanWon, Yo SeobChoi, Soo HoKim, Jae WooAdofo, Laud AnimKim, Soo MinKim, Ki Kang
DOI
10.1039/d3cc01510f
발행일
2023-07
유형
Article
저널명
Chemical Communications
59
60
페이지
9247 ~ 9250