Enzymatic Synthesis of Structured Monogalactosyldiacylglycerols Enriched in Pinolenic Acid
  • Kim, Jiwon
  • Chung, Min-Yu
  • Choi, Hee-Don
  • Choi, In-Wook
  • Kim, Byung Hee
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초록

We enzymatically prepared structured monogalactosydiacylglycerols (MGDGs) enriched in pinolenic acid (PLA). PLA-enriched free fatty acids (FFAs) containing similar to 86 mol % PLA were produced from an FFA fraction obtained from pine nut oil (PLA content, similar to 13 mol %) by urea crystallization. Commercial MGDGs (5 mg) were acidolyzed with PLA-enriched FFAs using four commercial immobilized lipases as biocatalysts. The reaction was performed in acetone (4 mL) in a stirred-batch reactor. Lipozyme RM IM (immobilized Rhizomucor miehei lipase) was the most effective biocatalyst for the reaction. Structured MGDGs containing 42.1 mol % PLA were obtained under optimal reaction conditions: temperature, 25 degrees C; substrate molar ratio, 1:30 (MGDGs/PLA-enriched FFAs); enzyme loading, 20 wt % of total substrates; and reaction time, 36 h. The structured MGDGs were separated from the reaction products at a purity of 96.6 wt % using silica column chromatography. The structured MGDGs could be possibly used as emulsifiers with appetite-suppression effects.

키워드

acidolysisappetite suppressantsemulsifiersLipozyme RM IMmonogalactosyldiacylglycerolspinolenic acidstructured lipidsLIPASE-CATALYZED ACIDOLYSISPINE NUT OILTRIACYLGLYCEROLSESTERIFICATIONLIPIDS
제목
Enzymatic Synthesis of Structured Monogalactosyldiacylglycerols Enriched in Pinolenic Acid
저자
Kim, JiwonChung, Min-YuChoi, Hee-DonChoi, In-WookKim, Byung Hee
DOI
10.1021/acs.jafc.8b02599
발행일
2018-08
유형
Article
저널명
Journal of Agricultural and Food Chemistry
66
30
페이지
8079 ~ 8085