Iron/carbon composite microfiber catalyst derived from hemoglobin blood protein for lithium-oxygen batteries
  • Lee, Jun-Seo
  • Kim, Hyun-Soo
  • Ryu, Won-Hee
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초록

Recycling of bio-waste sources for synthesis of functional electrode materials is an eco-friendly and sustainable approach to realize next-generation energy-storage systems. In this study, we present a fabrication method of Fe/C composite microfibers derived from electrospinning of hemoglobin blood protein, and subsequent calcination, and investigate its functionality as an oxygen electrode catalyst for Li-O-2 batteries. We elucidate the thermal decomposition behavior of raw hemoglobin protein and structural evolution after calcination at different temperatures. We successfully fabricated Fe/C composite microfibers with a uniform and flattened shape by electrospinning of a hemoglobin precursor and thermal treatment. Finally, we demonstrated that Li-O-2 cells in which the Fe/C composite microfiber catalyst was incorporated in the oxygen electrodes exhibited improved electrochemical performance compared to a pristine reference cell without the catalyst.

키워드

Lithium-oxygen batteryHemoglobinIron/carbon compositeCatalystElectrospinningBlood proteinREDOX MEDIATORELECTROLYTENANOFIBERSAIRNANOPARTICLESNANOFLAKESREDUCTIONEVOLUTIONCAPACITYDESIGN
제목
Iron/carbon composite microfiber catalyst derived from hemoglobin blood protein for lithium-oxygen batteries
저자
Lee, Jun-SeoKim, Hyun-SooRyu, Won-Hee
DOI
10.1016/j.apsusc.2018.10.023
발행일
2019-02
유형
Article
저널명
Applied Surface Science
466
페이지
562 ~ 567