Synthesis of Quinoline-Indole Hybrids through Cu(II)-Catalyzed Amination and Annulation between <i>N</i>-Oxides and <i>o</i>-Alkynylanilines
  • Rakshit, Amitava
  • Moon, Kyeongwon
  • Singh, Pargat
  • Park, Jung Su
  • Kim, In Su
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초록

The synthesis of (iso)quinoline-indole hybrids by reacting (iso)quinoline N-oxides with o-alkynylanilines in the presence of a combination of copper(II) catalyst and a bidentate 2,2 '-bipyridine ligand is described. The utility of this method was demonstrated through site-selective functionalization of the synthesized products. A plausible reaction pathway for site-selective amination followed by annulative indole formation was elucidated by a series of mechanistic investigations.

키워드

CROSS-COUPLING REACTIONSBOND FORMATIONC-NCASCADE ANNULATIONH ACTIVATIONPALLADIUM
제목
Synthesis of Quinoline-Indole Hybrids through Cu(II)-Catalyzed Amination and Annulation between <i>N</i>-Oxides and <i>o</i>-Alkynylanilines
저자
Rakshit, AmitavaMoon, KyeongwonSingh, PargatPark, Jung SuKim, In Su
DOI
10.1021/acs.orglett.4c04375
발행일
2024-12
유형
Article
저널명
Organic Letters
26
51
페이지
11218 ~ 11223