Photocatalysis of Cr- and Fe-Doped CeO2 Nanoparticles to Selective Oxidation of 5-Hydroxymethylfurfural
  • Nam, Jeong-Woo
  • Pham, Vy Ngoc
  • Ha, Jeong Min
  • Shin, Minjeong
  • Lee, Hangil
  • 외 1명
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초록

Oxygen vacancies (Vo) present in CeO2 nanoparticles (NPs) can effectively boost their photocatalytic activity under ultraviolet (UV) light. To improve photocatalytic performance, Cr- and Fe-doped CeO2 NPs with increased Vo were prepared using a simple method of doping Cr and Fe ions into CeO2 NPs, which was confirmed by an in-depth analysis of the structural and electronic changes. Through photocatalytic degradation (PCD) experiments with 5-hydroxymethylfurfural (HMF), we found that the PCD rates of the two doped CeO2 NPs were faster than that of the CeO2 NPs. In addition, the conversion of HMF to 2,5-furandicarboxylic acid (FDCA) using the doped CeO2 NPs occurred only through the mechanism of the selective oxidation to 5-hydroxymethyl-2-furancarboxylic acid (HMFCA), exhibiting better efficiency than using CeO2 NPs. © 2022 by the authors.

키워드

5-hydroxymethylfurfuraloxygen vacancyphotocatalytic propertytransition metal-doped CeO2 nanoparticles2,5-FURANDICARBOXYLIC ACIDHETEROGENEOUS CATALYSTSOXYGEN VACANCIESDEFECT STRUCTURECO OXIDATIONCERIACHEMISTRYNANOSHEETSINTERFACE
제목
Photocatalysis of Cr- and Fe-Doped CeO2 Nanoparticles to Selective Oxidation of 5-Hydroxymethylfurfural
저자
Nam, Jeong-WooPham, Vy NgocHa, Jeong MinShin, MinjeongLee, HangilYoun, Young-Sang
DOI
10.3390/nano13010044
발행일
2023-01
유형
Article
저널명
Nanomaterials
13
1