Atomic sawtooth-like metal films for vdW-layered single-crystal growth
DC Field | Value | Language |
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dc.contributor.author | Ko, Hayoung | - |
dc.contributor.author | Choi, Soo Ho | - |
dc.contributor.author | Park, Yunjae | - |
dc.contributor.author | Lee, Seungjin | - |
dc.contributor.author | Oh, Chang Seok | - |
dc.contributor.author | Kim, Sung Youb | - |
dc.contributor.author | Lee, Young Hee | - |
dc.contributor.author | Kim, Soo Min | - |
dc.contributor.author | Ding, Feng | - |
dc.contributor.author | Kim, Ki Kang | - |
dc.date.accessioned | 2024-08-06T03:00:45Z | - |
dc.date.available | 2024-08-06T03:00:45Z | - |
dc.date.issued | 2024-07 | - |
dc.identifier.issn | 2041-1723 | - |
dc.identifier.issn | 2041-1723 | - |
dc.identifier.uri | https://scholarworks.sookmyung.ac.kr/handle/2020.sw.sookmyung/160340 | - |
dc.description.abstract | Atomic sawtooth surfaces have emerged as a versatile platform for growth of single-crystal van der Waals layered materials. However, the mechanism governing the formation of single-crystal atomic sawtooth metal (copper or gold) films on hard substrates (tungsten or molybdenum) remains a puzzle. In this study, we aim to elucidate the formation mechanism of atomic sawtooth metal films during melting-solidification process. Utilizing molecular dynamics, we unveil that the solidification of the liquid copper initiates at a high-index tungsten facet with higher interfacial energy. Subsequent tungsten facets follow energetically favourable pathways of forming single-crystal atomic sawtooth copper film during the solidification process near melting temperature. Formation of atomic sawtooth copper film is guaranteed with a film thickness exceeding the grain size of polycrystalline tungsten substrate. We further demonstrate the successful growth of centimeter-scale single-crystal monolayer hexagonal boron nitride films on atomic sawtooth copper films and explore their potential as efficient oxygen barrier. Although single-crystal (SC) 2D materials can be grown on atomic sawtooth metal surfaces, the formation mechanism during the melting-solidification process remains unclear. Here authors reveal that solidification starts at high-index facets and spreads, forming a SC atomic sawtooth surface. | - |
dc.language | 영어 | - |
dc.language.iso | ENG | - |
dc.publisher | NATURE PORTFOLIO | - |
dc.title | Atomic sawtooth-like metal films for vdW-layered single-crystal growth | - |
dc.type | Article | - |
dc.publisher.location | 독일 | - |
dc.identifier.doi | 10.1038/s41467-024-50184-5 | - |
dc.identifier.scopusid | 2-s2.0-85198094115 | - |
dc.identifier.wosid | 001266702400021 | - |
dc.identifier.bibliographicCitation | NATURE COMMUNICATIONS, v.15, no.1 | - |
dc.citation.title | NATURE COMMUNICATIONS | - |
dc.citation.volume | 15 | - |
dc.citation.number | 1 | - |
dc.type.docType | Article | - |
dc.description.isOpenAccess | Y | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.relation.journalWebOfScienceCategory | Multidisciplinary Sciences | - |
dc.subject.keywordPlus | HEXAGONAL BORON-NITRIDE | - |
dc.subject.keywordPlus | MONOLAYER | - |
dc.subject.keywordPlus | GRAPHENE | - |
dc.identifier.url | https://www.researchgate.net/publication/382177994_Atomic_sawtooth-like_metal_films_for_vdW-layered_single-crystal_growth | - |
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