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Achieving One-Electron Oxidation of a Mononuclear Nonheme Iron(V)-Imido Complex

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dc.contributor.authorHong, Seungwoo-
dc.contributor.authorLu, Xiaoyan-
dc.contributor.authorLee, Yong-Min-
dc.contributor.authorSeo, Mi Sook-
dc.contributor.authorOhta, Takehiro-
dc.contributor.authorOgura, Takashi-
dc.contributor.authorClemancey, Martin-
dc.contributor.authorMaldivi, Pascale-
dc.contributor.authorLatour, Jean-Marc-
dc.contributor.authorSarangi, Ritimukta-
dc.contributor.authorNam, Wonwoo-
dc.date.available2021-02-22T11:11:41Z-
dc.date.issued2017-10-
dc.identifier.issn0002-7863-
dc.identifier.issn1520-5126-
dc.identifier.urihttps://scholarworks.sookmyung.ac.kr/handle/2020.sw.sookmyung/8113-
dc.description.abstractA mononuclear nonheme iron(V)-imido complex, earing a tetraamido macrocyclic ligand (TAML), [Fe-V(NTs)(TAIVIL)](-) (1), was oxidized by one-electron oxidants, affording formation,of an iron(V)-imido TAML cation radical species; [Fe-V(NTs)(TAML(+.))] (2); 2 is a diamagnetic (S = 0) complex, resulting froni the antiferroinagnetic coupling of the low-spin iron(V) ion (S = 1/2) with the one-electron oxidized ligand (TAML(+)). 2 is a competent oxidant in C-H bond functionalization and riltrene transfer reaction, showing that the reactivity of 2 is greater than that of 1.-
dc.format.extent4-
dc.language영어-
dc.language.isoENG-
dc.publisherAMER CHEMICAL SOC-
dc.titleAchieving One-Electron Oxidation of a Mononuclear Nonheme Iron(V)-Imido Complex-
dc.typeArticle-
dc.publisher.location미국-
dc.identifier.doi10.1021/jacs.7b08161-
dc.identifier.scopusid2-s2.0-85031759744-
dc.identifier.wosid000413503300011-
dc.identifier.bibliographicCitationJOURNAL OF THE AMERICAN CHEMICAL SOCIETY, v.139, no.41, pp 14372 - 14375-
dc.citation.titleJOURNAL OF THE AMERICAN CHEMICAL SOCIETY-
dc.citation.volume139-
dc.citation.number41-
dc.citation.startPage14372-
dc.citation.endPage14375-
dc.type.docTypeArticle-
dc.description.isOpenAccessN-
dc.description.journalRegisteredClasssci-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.relation.journalResearchAreaChemistry-
dc.relation.journalWebOfScienceCategoryChemistry, Multidisciplinary-
dc.subject.keywordPlusTRANSITION-METAL-COMPLEXES-
dc.subject.keywordPlusHIGH-VALENT IRON-
dc.subject.keywordPlusATOM-TRANSFER-
dc.subject.keywordPlusREACTIVITY-
dc.subject.keywordPlusMECHANISMS-
dc.subject.keywordPlusCHEMISTRY-
dc.subject.keywordPlusOXO-
dc.subject.keywordPlusSPECTROSCOPY-
dc.subject.keywordPlusIRON(IV)-OXO-
dc.subject.keywordPlusOXAZOLINE-
dc.identifier.urlhttps://pubs.acs.org/doi/10.1021/jacs.7b08161-
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