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Reactivity comparison of high-valent iron(IV)-oxo complexes bearing N-tetramethylated cyclam ligands with different ring size
- Authors
- Hong, S (Hong, Seungwoo); So, H (So, Hee); Yoon, H (Yoon, Heejung); Cho, KB (Cho, Kyung-Bin); Lee, YM (Lee, Yong-Min); Fukuzumi, S (Fukuzumi, Shunich; Nam, W (Nam, Wonwoo)
- Issue Date
- Jun-2013
- Publisher
- ROYAL SOC CHEMISTRY
- Citation
- DALTON TRANSACTIONS, v.42, no.22, pp 7842 - 7845
- Pages
- 4
- Journal Title
- DALTON TRANSACTIONS
- Volume
- 42
- Number
- 22
- Start Page
- 7842
- End Page
- 7845
- ISSN
- 1477-9226
1477-9234
- Abstract
- The ring size effect of macrocyclic TMC ligands in nonheme iron(IV)-oxo complexes has been examined in hydrogen atom transfer (HAT) and oxygen atom transfer (OAT) reactions; an iron(IV)-oxo complex bearing a smaller TMC ligand is more reactive in both HAT and OAT reactions, resulting from its high Fe-IV/III redox potential.
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