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Dual Role of Anthranils as Amination and Transient Directing Group Sources: Synthesis of 2-Acyl Acridines
- Authors
- Kim, Saegun; Han, Sang Hoon; Mishra, Neeraj Kumar; Chun, Rina; Jung, Young Hoon; Kim, Hyung Sik; Park, Jung Su; Kim, In Su
- Issue Date
- Jul-2018
- Publisher
- AMER CHEMICAL SOC
- Citation
- ORGANIC LETTERS, v.20, no.13, pp 4010 - 4014
- Pages
- 5
- Journal Title
- ORGANIC LETTERS
- Volume
- 20
- Number
- 13
- Start Page
- 4010
- End Page
- 4014
- ISSN
- 1523-7060
1523-7052
- Abstract
- The transient directing group promoted C-(sp(2))-H functionalization of benzaldehydes with anthranils by a cationic rhodium(III) catalyst is described. Notably, anthranils have been used as both transient directing groups and amination sources to afford 2-aryl acridines through direct C-H amination followed by acid-mediated cyclization. A range of substrate scopes and functional group tolerance were observed.
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